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Bimodality in the knotting probability of semiflexible rings suggested by mapping with self-avoiding polygons

Uehara, Erica
•
Coronel, Lucia
•
Micheletti, Cristian
•
Deguchi, Tetsuo
2019
  • journal article

Periodico
REACTIVE & FUNCTIONAL POLYMERS
Abstract
We use a simple physical mapping to adapt the known asymptotic expressions for the knotting probabilities ofself-avoiding polygons to the case of semiflexible rings of beads. We thus obtain analytical expressions thatapproximate the abundance of the simplest knots as a function of the length and bending rigidity of the rings. Wevalidate the predictions against previously published data from stochastic simulations of rings of beads showingthat they reproduce the intriguing non-monotonic dependence of knotting probability on bending rigidity. Themapping thus provides a useful theoretical tool not only for a physically-transparent interpretation of previousresults, but especially to predict the knotting probabilities for previously unexplored combinations of chainlengths and bending rigidities. In particular, our mapping suggests that for rings longer than 20,000 beads, therigidity-dependent knotting probability profile switches from unimodal to bimodal
DOI
10.1016/j.reactfunctpolym.2018.11.008
WOS
WOS:000456903200016
Archivio
http://hdl.handle.net/20.500.11767/85902
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85057482781
https://www.sciencedirect.com/science/article/pii/S1381514818310174?via%3Dihub
Diritti
closed access
Soggetti
  • knots

  • Knotting probability

  • Settore FIS/03 - Fisi...

Scopus© citazioni
5
Data di acquisizione
Jun 7, 2022
Vedi dettagli
Web of Science© citazioni
6
Data di acquisizione
Mar 27, 2024
Visualizzazioni
4
Data di acquisizione
Apr 19, 2024
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