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Photoemission study of twisted monolayers and bilayers of WSe2 on graphite substrates

Parashar B.
•
Rathmann L.
•
Kim H. -J.
altro
Plucinski L.
2023
  • journal article

Periodico
PHYSICAL REVIEW MATERIALS
Abstract
Using microfocused angle-resolved photoemission spectroscopy we investigated microstructures containing regions of single-layer (SL) and bilayer (BL) WSe2 on graphite substrates at different twist angles between SL WSe2 and graphite and within the BL WSe2. Fermi level electrons emitted from the graphite are sharply focused near their Kgr points in the Brillouin zone, and, when passing through the WSe2, get diffracted to form band replicas readily observed in experimental Fermi surface maps from twisted SL WSe2/graphite. We investigated two twisted BL WSe2 at twist angles ∼28° and ∼10° and found no evidence of hybridization gaps at the interlayer band-crossing points, that could be precursors of the flat bands at smaller twist angles. Similarly, no such gaps were found for SL WSe2/graphite. Experimental results are complemented by theoretical density functional theory calculations, which suggest that a formation of hybridization gaps in the WSe2/graphene (which approximates the experimental WSe2/graphite system) sensitively depends on the WSe2 band character at the crossing point with the graphene Dirac band.
DOI
10.1103/PhysRevMaterials.7.044004
WOS
WOS:000973461700002
Archivio
https://hdl.handle.net/11368/3067392
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85153531325
https://journals.aps.org/prmaterials/abstract/10.1103/PhysRevMaterials.7.044004
Diritti
open access
license:copyright editore
license:copyright editore
license uri:iris.pri02
license uri:iris.pri02
FVG url
https://arts.units.it/bitstream/11368/3067392/2/PhysRevMaterials.7.044004.pdf
Soggetti
  • TMD

  • Graphene

  • ARPES

  • Twist

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