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Attosecond electronic and nuclear quantum photodynamics of ozone monitored with time and angle resolved photoelectron spectra

DECLEVA, PIETRO
•
QUADRI, NICOLA
•
Perveaux, Aurelie
altro
Vibók, à gnes
2016
  • journal article

Periodico
SCIENTIFIC REPORTS
Abstract
Recently we reported a series of numerical simulations proving that it is possible in principle to create an electronic wave packet and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few femtoseconds. We considered the ozone molecule: for this system the electronic wave packet leads to a dissociation process. In the present work, we investigate more specifically the time-resolved photoelectron angular distribution of the ozone molecule that provides a much more detailed description of the evolution of the electronic wave packet. We thus show that this experimental technique should be able to give access to observing in real time the creation of an electronic wave packet in a neutral molecule and its impact on a chemical process.
DOI
10.1038/srep36613
WOS
WOS:000387068800001
Archivio
http://hdl.handle.net/11368/2902609
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-84994387511
https://www.nature.com/articles/srep36613
Diritti
open access
license:creative commons
license uri:http://creativecommons.org/licenses/by/3.0/it/
FVG url
https://arts.units.it/bitstream/11368/2902609/2/srep36613.pdf
Soggetti
  • Multidisciplinary

Scopus© citazioni
3
Data di acquisizione
Jun 14, 2022
Vedi dettagli
Web of Science© citazioni
4
Data di acquisizione
Mar 27, 2024
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