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Inhomogeneous disordering at a photoinduced charge density wave transition

Picano, Antonio
•
Grandi, Francesco
•
Eckstein, Martin
2023
  • journal article

Periodico
PHYSICAL REVIEW. B
Abstract
Using ultrashort laser pulses, it has become possible to probe the dynamics of long-range order in solids on microscopic timescales. In the conventional description of symmetry-broken phases within time-dependent Ginzburg-Landau theory, the order parameter evolves coherently, with small fluctuations along an average trajec-tory. Recent experiments, however, indicate that some systems can support a different scenario, named ultrafast inhomogeneous disordering, where the average order parameter is no longer representative of the state on the atomic scale. Here we theoretically show that ultrafast disordering can occur in a minimal, yet paradigmatic, model for a Peierls instability if atomic scale inhomogeneities of both the electronic structure and the charge density wave order parameter are taken into account. The latter is achieved using a nonequilibrium generalization of statistical dynamical mean-field theory coupled to stochastic differential equations for the order parameter.
DOI
10.1103/physrevb.107.245112
WOS
WOS:001015589300002
Archivio
https://hdl.handle.net/20.500.11767/142130
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85161907970
https://ricerca.unityfvg.it/handle/20.500.11767/142130
Diritti
closed access
google-scholar
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