Active control of wrinkling in soft film-substrate composites using electric fields is a critical challenge in tunable material systems. Here, we investigate the electro-mechanical instability of a soft dielectric film bonded to a hyperelastic substrate, revealing the fundamental mechanisms that enable on-demand surface patterning. For the linearized stability analysis, we use the Stroh formalism and the surface impedance method to obtain exact and sixth-order approximate bifurcation equations that signal the onset of wrinkles. We derive the explicit bifurcation equations giving the critical stretch and critical voltage for wrinkling, as well as the corresponding critical wavenumber. We look at scenarios where the voltage is kept constant and the stretch changes, and vice versa. We provide the thresholds of the shear modulus ratio rc0 or pre-stretch λc0 below which the film-substrate system wrinkles mechanically, prior to the application of a voltage. These predictions offer theoretical guidance for practical structural design, as the shear modulus ratio r and/or the pre-stretch λ can be chosen to be slightly greater than rc0 and/or λc0, so that the film-substrate system wrinkles with a small applied voltage. Finally, we simulate the full nonlinear behavior using the Finite Element method (FEniCS) to validate our formulas and conduct a post-buckling analysis. This work advances the fundamental understanding of electro-mechanical wrinkling instabilities in soft material systems. By enabling active control of surface morphologies via applied electric fields, our findings open new avenues for adaptive technologies in soft robotics, flexible electronics, smart surfaces, and bioinspired systems.
