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Ultrafast all-optical manipulation of the charge-density wave in VTe2

Tuniz, Manuel
•
Soranzio, Davide
•
Bidoggia, Davide
altro
Cilento, Federico
2023
  • journal article

Periodico
PHYSICAL REVIEW RESEARCH
Abstract
The charge-density-wave (CDW) phase in the layered transition-metal dichalcogenide VTe2 is strongly coupled to the band inversion involving vanadium and tellurium orbitals. In particular, this coupling leads to a selective disappearance of the Dirac-type states that characterize the normal phase, when the CDW phase sets in. Here, we investigate the broadband time-resolved reflectivity variations caused by collective and single-particle excitations in the CDW ground state of VTe2. With the aid of density functional perturbation theory simulations we unveil the presence of two collective amplitude modes of the CDW ground state. By applying a double-pulse excitation scheme, we show the possibility to manipulate these modes, gaining insights into the coupling between these two collective excitations and demonstrating a more efficient way to perturb the CDW phase in VTe2.
DOI
10.1103/physrevresearch.5.043276
WOS
WOS:001133312500002
Archivio
https://hdl.handle.net/11368/3070298
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85180993563
https://journals.aps.org/prresearch/abstract/10.1103/PhysRevResearch.5.043276
Diritti
open access
license:creative commons
license:creative commons
license uri:http://creativecommons.org/licenses/by/4.0/
license uri:http://creativecommons.org/licenses/by/4.0/
FVG url
https://arts.units.it/bitstream/11368/3070298/1/PhysRevResearch.5.043276.pdf
Soggetti
  • Charge density wave

  • first principles calc...

  • transition metal dich...

  • topological material

  • ultrafast optics

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