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Pump-probe experiments at the TEMPO beamline using the low-α operation mode of Synchrotron SOLEIL

Silly M. G.
•
Ferte T.
•
Tordeux M. A.
altro
Cautero G.
2017
  • journal article

Periodico
JOURNAL OF SYNCHROTRON RADIATION
Abstract
The SOLEIL synchrotron radiation source is regularly operated in special filling modes dedicated to pump-probe experiments. Among others, the low-α mode operation is characterized by shorter pulse duration and represents the natural bridge between 50ps synchrotron pulses and femtosecond experiments. Here, the capabilities in low-α mode of the experimental set-ups developed at the TEMPO beamline to perform pump-probe experiments with soft X-rays based on photoelectron or photon detection are presented. A 282kHz repetition-rate femtosecond laser is synchronized with the synchrotron radiation time structure to induce fast electronic and/or magnetic excitations. Detection is performed using a two-dimensional space resolution plus time resolution detector based on microchannel plates equipped with a delay line. Results of time-resolved photoelectron spectroscopy, circular dichroism and magnetic scattering experiments are reported, and their respective advantages and limitations in the framework of high-time-resolution pump-probe experiments compared and discussed.The low-α operation mode of SOLEIL is presented and gives the operation details for experiments using soft X-rays at the TEMPO beamline. Experiments are presented to give the reader the possibility to evaluate the performances of the installation. With the increasing research activity using time-resolved experiments it should be interesting for the synchrotron radiation community. It is thought that the low-α mode operation is the natural bridge between the usual time scale of synchrotron pulses and laser-driven femtosecond experiments
DOI
10.1107/S1600577517007913
WOS
WOS:000404629100019
Archivio
http://hdl.handle.net/11368/2954998
info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-85021770295
https://onlinelibrary.wiley.com/doi/pdf/10.1107/S1600577517007913
Diritti
closed access
license:copyright editore
FVG url
https://arts.units.it/request-item?handle=11368/2954998
Soggetti
  • pump-probe experiment...

  • time-resolved spectro...

Web of Science© citazioni
15
Data di acquisizione
Mar 26, 2024
Visualizzazioni
2
Data di acquisizione
Apr 19, 2024
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